Nav: Home

Physicists propose perfect material for lasers

May 08, 2019

Weyl semimetals are a recently discovered class of materials, in which charge carriers behave the way electrons and positrons do in particle accelerators. Researchers from the Moscow Institute of Physics and Technology and Ioffe Institute in St. Petersburg have shown that these materials represent perfect gain media for lasers. The research findings were published in Physical Review B.

The 21st-century physics is marked by the search for phenomena from the world of fundamental particles in tabletop materials. In some crystals, electrons move as high-energy particles in accelerators. In others, particles even have properties somewhat similar to black hole matter.

MIPT physicists have turned this search inside-out, proving that reactions forbidden for elementary particles can also be forbidden in the crystalline materials known as Weyl semimetals. Specifically, this applies to the forbidden reaction of mutual particle-antiparticle annihilation without light emission. This property suggests that a Weyl semimetal could be the perfect gain medium for lasers.

In a semiconductor laser, radiation results from the mutual annihilation of electrons and the positive charge carriers called holes. However, light emission is just one possible outcome of an electron-hole pair collision. Alternatively, the energy can build up the oscillations of atoms nearby or heat the neighboring electrons. The latter process is called Auger recombination, in honor of the French physicist Pierre Auger (pronounced oh-ZHAY').

Auger recombination limits the efficiency of modern lasers in the visible and infrared range, and severely undermines terahertz lasers. It eats up electron-hole pairs that might have otherwise produced radiation. Moreover, this process heats up the device.

For almost a century, researchers have sought a "wonder material" in which radiative recombination dominates over Auger recombination. This search was guided by an idea formulated in 1928 by Paul Dirac. He developed a theory that the electron, which had already been discovered, had a positively charged twin particle, the positron. Four years later, the prediction was proved experimentally. In Dirac's calculations, a mutual annihilation of an electron and positron always produces light and can not impart energy on other electrons. This is why the quest for a wonder material to be used in lasers was largely seen as a search for analogues of the Dirac electron and positron in semiconductors.

"In the 1970s, the hopes were largely associated with lead salts, and in the 2000s - with graphene," says Dmitry Svintsov, the head of the Laboratory of 2D Materials for Optoelectronics at MIPT. "But the particles in these materials exhibited deviations from Dirac's concept. The graphene case proved quite pathological, because confining electrons and holes to two dimensions actually gives rise to Auger recombination. In the 2D world, there is little space for particles to avoid collisions."

"Our latest paper shows that Weyl semimetals are the closest we've gotten to realizing an analogy with Dirac's electrons and positrons," added Svintsov, who was the principal investigator in the reported study.

Electrons and holes in a semiconductor do have the same electric charges as Dirac's particles. But it takes more than that to eliminate Auger recombination. Laser engineers seek the kind of particles that would match Dirac's theory in terms of their dispersion relations. The latter tie particle's kinetic energy to its momentum. That equation encodes all the information on particle's motion and the reactions it can undergo.

In classical mechanics, objects such as rocks, planets, or spaceships follow a quadratic dispersion equation. That is, doubling of the momentum results in four-fold increase in kinetic energy. In conventional semiconductors -- silicon, germanium, or gallium arsenide -- the dispersion relation is also quadratic. For photons, the quanta of light, the dispersion relation is linear. One of the consequences is that a photon always moves at precisely the speed of light.

The electrons and positrons in Dirac's theory occupy a middle ground between rocks and photons: at low energies, their dispersion relation is quadratic, but at higher energies it becomes linear. Until recently, though, it took a particle accelerator to "catapult" an electron into the linear section of the dispersion relation.

Some newly discovered materials can serve as "pocket accelerators" for charged particles. Among them are the "pencil-tip accelerator" - graphene and its three-dimensional analogues, known as Weyl semimetals: tantalum arsenide, niobium phosphate, molybdenum telluride. In these materials, electrons obey a linear dispersion relation starting from the lowest energies. That is, the charge carriers behave like electrically charged photons. These particles may be viewed as analogous to the Dirac electron and positron, except that their mass approaches zero.

The researchers have shown that despite the zero mass, Auger recombination still remains forbidden in Weyl semimetals. Foreseeing the objection that a dispersion relation in an actual crystal is never strictly linear, the team went on to calculate the probability of "residual" Auger recombination due to deviations from the linear law. This probability, which depends on electron concentration, can reach values some 10,000 times lower than in the currently used semiconductors. In other words, the calculations suggest that Dirac's concept is rather faithfully reproduced in Weyl semimetals.

"We were aware of the bitter experience of our predecessors who hoped to reproduce Dirac's dispersion relation in real crystals to the letter," Svintsov explained. "That is why we did our best to identify every possible loophole for potential Auger recombination in Weyl semimetals. For example, in an actual Weyl semimetal, there exist several sorts of electrons, slow and fast ones. While a slower electron and a slower hole may collapse, the faster ones can pick up energy. That said, we calculated that the odds of that happening are low."

The team gauged the lifetime of an electron-hole pair in a Weyl semimetal to be about 10 nanoseconds. That timespan looks extremely small by everyday standards, but for laser physics, it is huge. In conventional materials used in laser technology of the far infrared range, the lifetimes of electrons and holes are thousands of times shorter. Extending the lifetime of nonequilibrium electrons and holes in novel materials opens up prospects for using them in new types of long-wavelength lasers.
-end-
Original research paper: Relativistic suppression of Auger recombination in Weyl semimetals; A. N. Afanasiev, A. A. Greshnov, and D. Svintsov; Phys. Rev. B 99, 115202 -- published March 4, 2019

Moscow Institute of Physics and Technology

Related Electrons Articles:

Deceleration of runaway electrons paves the way for fusion power
Fusion power has the potential to provide clean and safe energy that is free from carbon dioxide emissions.
Shining light on low-energy electrons
The classic method for studying how electrons interact with matter is by analyzing their scattering through thin layers of a known substance.
Ultrafast nanophotonics: Turmoil in sluggish electrons' existence
An international team of physicists has monitored the scattering behavior of electrons in a non-conducting material in real-time.
NASA mission uncovers a dance of electrons in space
NASA's MMS mission studies how electrons spiral and dive around the planet in a complex dance dictated by the magnetic and electric fields, and a new study revealed a bizarre new type of motion exhibited by these electrons.
'Hot' electrons don't mind the gap
Rice University scientists discover that 'hot' electrons can create a photovoltage about a thousand times larger than ordinary temperature differences in nanoscale gaps in gold wires.
Electrons used to control ultrashort laser pulses
We may soon get better insight into the microcosm and the world of electrons.
Supercool electrons
Study of electron movement on helium may impact the future of quantum computing.
Two electrons go on a quantum walk and end up in a qudit
There is a variety of physical systems that can be used to implement a separate quantum bit, but significantly less research has been done into systems of several qubits or qudits.
Radiation that knocks electrons out and down, one after another
Researchers at Japan's Tohoku University are investigating novel ways by which electrons are knocked out of matter.
Controlling electrons in time and space
A new method has been developed to control electrons being emitted from metal tips.

Related Electrons Reading:

Best Science Podcasts 2019

We have hand picked the best science podcasts for 2019. Sit back and enjoy new science podcasts updated daily from your favorite science news services and scientists.
Now Playing: TED Radio Hour

Digital Manipulation
Technology has reshaped our lives in amazing ways. But at what cost? This hour, TED speakers reveal how what we see, read, believe — even how we vote — can be manipulated by the technology we use. Guests include journalist Carole Cadwalladr, consumer advocate Finn Myrstad, writer and marketing professor Scott Galloway, behavioral designer Nir Eyal, and computer graphics researcher Doug Roble.
Now Playing: Science for the People

#529 Do You Really Want to Find Out Who's Your Daddy?
At least some of you by now have probably spit into a tube and mailed it off to find out who your closest relatives are, where you might be from, and what terrible diseases might await you. But what exactly did you find out? And what did you give away? In this live panel at Awesome Con we bring in science writer Tina Saey to talk about all her DNA testing, and bioethicist Debra Mathews, to determine whether Tina should have done it at all. Related links: What FamilyTreeDNA sharing genetic data with police means for you Crime solvers embraced...